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Liu Ming, Fan Dejiang, Zheng Shiwen, Tian Yuan, Zhang Aibin. Tracking lead origins in the central Bohai Sea based on stable lead isotope composition[J]. Haiyang Xuebao, 2016, 38(2): 36-47. doi: 10.3969/j.issn.0253-4193.2016.02.004
Citation: Liu Ming, Fan Dejiang, Zheng Shiwen, Tian Yuan, Zhang Aibin. Tracking lead origins in the central Bohai Sea based on stable lead isotope composition[J]. Haiyang Xuebao, 2016, 38(2): 36-47. doi: 10.3969/j.issn.0253-4193.2016.02.004

Tracking lead origins in the central Bohai Sea based on stable lead isotope composition

doi: 10.3969/j.issn.0253-4193.2016.02.004
  • Received Date: 2015-10-16
  • Rev Recd Date: 2015-11-27
  • The Pb concentration and stable isotopes (204Pb, 206Pb, 207Pb, and 208Pb) in surface and core sediments from the central Bohai Sea have been determined to investigate their spatial/temporal distribution and sources in this area. Results showed that the contents of Pb in surface sediments varied from 14.54×10-6 to 59.42×10-6, which had higher level in the coastal Bohai Bay, nearby Huanghe River estuary and northeast of the study area. Pb isotope ratio of 207Pb/206Pb and 208Pb/206Pb varied from 0.834 1-0.848 9 and 2.082 8-2.098 0 in surface sediments, respectively. The core sediment records showed that Pb content and isotopic composition were similar to the surface sediments. However, the vertical values of Pb content and isotopic ratios were stable overall, but they presented an increasing trend since 1990s. Pb in the central Bohai Sea sediments were mainly origined from natural materials, and the Huanghe River substances was the dominated source, while the northern end of the Bohai Bay was affected by the Luanhe River or coastal erosion. The impact of human activities on the Pb deposition appeared since 1990s in the sedimentary records, which mainly referred to the combustion of Chinese leaded ores and other industrial activities. However, the impact was weak, only reflected on several sites in the northwest of Huanghe River mouth and Bohai Bay.
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