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冲绳海槽中南部柱状沉积物氧化还原敏感元素赋存机理与环境指示意义

许晓燕 窦衍光 张勇 陈晓辉 孙治雷 白凤龙 翟滨 王利波 邹亮

许晓燕,窦衍光,张勇,等. 冲绳海槽中南部柱状沉积物氧化还原敏感元素赋存机理与环境指示意义[J]. 海洋学报,2022,44(10):63–79 doi: 10.12284/hyxb2022186
引用本文: 许晓燕,窦衍光,张勇,等. 冲绳海槽中南部柱状沉积物氧化还原敏感元素赋存机理与环境指示意义[J]. 海洋学报,2022,44(10):63–79 doi: 10.12284/hyxb2022186
Xu Xiaoyan,Dou Yanguang,Zhang Yong, et al. Occurrence mechanism of redox sensitive elements in columnar sediments in South Central Okinawa Trough and their environmental implications[J]. Haiyang Xuebao,2022, 44(10):63–79 doi: 10.12284/hyxb2022186
Citation: Xu Xiaoyan,Dou Yanguang,Zhang Yong, et al. Occurrence mechanism of redox sensitive elements in columnar sediments in South Central Okinawa Trough and their environmental implications[J]. Haiyang Xuebao,2022, 44(10):63–79 doi: 10.12284/hyxb2022186

冲绳海槽中南部柱状沉积物氧化还原敏感元素赋存机理与环境指示意义

doi: 10.12284/hyxb2022186
基金项目: 国家自然科学基金(41776077);国家海洋局国际合作项目(GASI-GEOGEO-04);中国地质调查局地质调查专项(DD20190205,DD20221710)。
详细信息
    作者简介:

    许晓燕(1997-),女,广东省汕头市人,主要从事海洋地质研究。E-mail: 1114323281@qq.com

    通讯作者:

    窦衍光(1979-),男,研究员,主要从事海洋沉积地球化学研究。E-mail: douyangaung@gmail.com

  • 中图分类号: P736.4+1

Occurrence mechanism of redox sensitive elements in columnar sediments in South Central Okinawa Trough and their environmental implications

  • 摘要: 沉积物中氧化还原敏感元素(Redox Sensitive Element,RSE)含量变化是上覆水体氧化还原环境良好的替代指标。本文通过冲绳海槽中南部两个柱状沉积物(深度:30 cm)粒度、总有机碳、总氮及其同位素含量和氧化还原敏感元素含量等指标,探究复杂环境背景下冲绳海槽柱状沉积物中RSE的赋存机理与环境指示意义。研究发现,柱状沉积物中除了Cr亏损,其他RSE均显示有不同程度的富集。“粒控效应”对冲绳海槽柱状沉积物的RSE含量影响较小;分析可知,海水表层生产力是影响沉积物氧化还原环境的主要因素,通过Mn(氢)氧化物的吸附或解吸附作用实现RSE的富集与亏损。δCe、V/Cr、Ni/Co和V/(V+Ni)等指标指示沉积物整体处于氧化−弱氧化环境。沉积物中Mn元素通过还原作用以Mn2+形式向上扩散,在25~30 cm处被含氧间隙水氧化富集形成锰峰,指示柱状沉积物0~25 cm处为氧化环境,25~30 cm处为弱氧化环境。
  • 图  1  东海冲绳海槽洋流体系[31]及样品位置

    Fig.  1  Ocean current system[31] and sample location in the Okinawa Trough of the East China Sea

    图  2  DYBB27(a)和DYB228(b)柱状沉积物组分含量、平均粒径、TOC含量、TN含量、δ13C值、δ15N值和海洋自生有机质组分占比(fm)的垂向特征

    Fig.  2  Vertical characteristics of component content, average particle size, TOC content, TN content, δ13C value, δ15N value and fm in the columnar sediments of DYBB27 (a) and DYB228 (b)

    图  3  DYBB27和DYB228柱状沉积物中RSE/Al比值的垂向特征

    Fig.  3  Vertical characteristics of RSE/Al ratio in the columnar sediments of DYBB27 and DYB228

    图  4  DYBB27和DYB228柱状沉积物RSEEF的垂向特征

    Fig.  4  Vertical characteristics of RSEEF in the columnar sediments of DYBB27 and DYB228

    图  5  DYBB27和DYB228柱状沉积物不同氧化还原指标的变化特征(Uauth为自生铀含量)

    Fig.  5  Variation characteristics of different oxidation indicators in columnar sediments of DYBB27 and DYB228 (Uauth is the content of authigenic uranium)

    图  6  DYBB27(a)和DYB228(b)柱状沉积物中粉砂含量和RSE/Al比值的相关性

    纵坐标a值除了Mn/Al比值为1,其他RSE/Al比值为4

    Fig.  6  Correlation between silt content and RSE/Al ratios in the columnar sediments of DYBB27 (a) and DYB228 (b)

    The value of ordinate a is 1 (Mn/Al), and the other RSE/Al are 4

    图  7  DYBB27(深蓝色)和DYB228(蓝色)柱状沉积物中生源钡(Babio)与TOC含量和RSE/Al比值的相关性

    Fig.  7  Correlations of bio-barium (Babio) content with TOC content and RSE/Al ratios in the columnar sediments of DYBB27 (dark blue) and DYB228 (blue)

    图  8  DYBB27 (a)和DYB228 (b)柱状沉积物中Mn/Al比值和RSE/Al比值的相关性

    Fig.  8  Correlation of Mn/Al ratio and RSE/Al ratios in the columnar sediments of DYBB27 (a) and DYB228 (b)

    图  9  Babio含量和MnO/Al2O3比值的相关性

    Fig.  9  Correlations of Babio content and MnO/Al2O3 ratio

    图  10  DYBB27和DYB228柱状沉积物中Ni/Co和V/Cr比值分布

    其他数据引自文献[89]

    Fig.  10  Distribution of Ni/Co and V/Cr ratios in columnar sediments of DYBB27 and DYB228

    Other data are quoted from reference [89]

    图  11  DYBB27和DYB228柱状沉积物中V/(V+Ni) 和Mn/(Al×10) 比值的相关性

    Fig.  11  Correlation of V/(V+Ni) and Mn/(Al×10) ratios in columnar sediments of DYBB27 and DYB228

    表  1  冲绳海槽中南部不同钻孔沉积物的AMS14C测年数据对比

    Tab.  1  Comparison of AMS14C dating data of sediments from different drillings in the South Central Okinawa Trough

    样品编号纬度经度水深/m深度/cm距今平均校正年龄/(cal a)参考文献
    DYBB2726.196 9°N125.233 8°E1 32329~30140本研究
    DYB22826.866 3°N125.955 0°E1 27729~3067.5本研究
    MD01240426.656 7°N125.820 8°E1 39714.5749文献[39]
    OKT-326.018 0°N125.282 0°E1 792281 090文献[40]
    OKI-15126.110 0°N125.520 0°E2 013301 135文献[41]
    A727.817 2°N126.968 6°E1 26432~362 690文献[42]
    C1428.659 7°N127.320 0°E1 10035~37.5673文献[43]
    Oki0226.073 6°N125.200 7°E1 61252~542 891文献[44]
    OKT12-226.050 0°N125.340 0°E1 924.53573 147.5文献[45]
    下载: 导出CSV

    表  2  DYBB27和DYB228柱状沉积物RSE/Al比值与粒径的相关性分析

    Tab.  2  Correlation analysis of RSE/Al ratio and particle size in the columnar sediments of DYBB27 and DYB228

    样品指标U/AlV/AlCr/AlNi/AlCo/AlCu/AlFe/AlMn/Al
    DYBB27平均粒径−0.177−0.2830.067−0.0920.285−0.1140.140−0.079
    砂粒径0.442*0.281−0.0370.036−0.393*−0.005−0.384*−0.018
    粉砂粒径−0.607**−0.196−0.0530.0340.369*0.1980.539**0.129
    黏土粒径0.175−0.1250.114−0.0890.058−0.240−0.166−0.137
    DYB228平均粒径0.554**−0.198−0.416*−0.245−0.069−0.216−0.335−0.056
    砂粒径−0.1000.1280.016−0.203−0.240−0.1930.034−0.259
    粉粒粒径−0.440*0.0420.424*0.517**0.375*0.508**0.3400.390*
    黏土粒径0.748**−0.197−0.635**−0.538**−0.291−0.027−0.532**−0.293
    注:**表示在0.01级别(双尾),相关性显著;*表示在0.05级别(双尾),相关性显著。
    下载: 导出CSV

    表  3  DYBB27和DYB228柱状沉积物RSE/Al比值与TOC和Babio的相关性分析

    Tab.  3  Correlation analysis of RSE/Al ratios with TOC and BaBio in the columnar sediments of DYBB27 and DYB228

    样品指标Babio含量/10−6U/AlV/AlCr/AlNi/AlCo/AlCu/Al
    DYBB27TOC含量/%0.147−0.093−0.014−0.0530.1000.182−0.036
    Babio含量/10−61−0.0170.686**0387*0.844**0.749**0.248
    DYB228TOC含量/%0.206−0.427*0.501**0.1950.0390.3600.447*
    Babio含量/10−61−0.282−0.3120.0680.759**0.858**0.383*
    注:**表示在0.01级别(双尾),相关性显著;*表示在0.05级别(双尾),相关性显著。
    下载: 导出CSV

    表  4  DYBB27和DYB228柱状沉积物RSE/Al比值与Fe/Al和Mn/Al比值的相关性分析

    Tab.  4  Correlation analysis of RSE/Al ratios with Fe/Al and Mn/Al ratios in the columnar sediments of DYBB27 and DYB228

    站位指标U/AlV/AlCr/AlNi/AlCo/AlCu/Al
    DYBB27Fe/Al−0.677**−0.181−0.006−0.1260.0320.053
    Mn/Al−0.2480.666**0.2740.972**0.821**0.361
    DYB228Fe/Al−0.672**0.391*0.442*0.153−0.1390.299
    Mn/Al−0.333−0.2290.0890.896**0.901**0.529**
    注:**表示在0.01级别(双尾),相关性显著;*表示在0.05级别(双尾),相关性显著。
    下载: 导出CSV
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  • 收稿日期:  2022-02-09
  • 修回日期:  2022-06-22
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