Message Board

Respected readers, authors and reviewers, you can add comments to this page on any questions about the contribution, review, editing and publication of this journal. We will give you an answer as soon as possible. Thank you for your support!

Full name
E-mail
Phone number
Title
Message
Verification Code
Zhou Peiyu, Chen Changshu, Hu Ping, Ye Jianjun, Shangguan Maosen, Liu Jingqin, Wu Lingling, Fang Hongda, Huang Chuguang. Oil fingerprinting of polyaromatic hydrocarbons applied to the identification study of oil spill from ship[J]. Haiyang Xuebao, 2014, 36(12): 91-102. doi: 10.3969/j.issn.0253-4193.2014.12.009
Citation: Zhou Peiyu, Chen Changshu, Hu Ping, Ye Jianjun, Shangguan Maosen, Liu Jingqin, Wu Lingling, Fang Hongda, Huang Chuguang. Oil fingerprinting of polyaromatic hydrocarbons applied to the identification study of oil spill from ship[J]. Haiyang Xuebao, 2014, 36(12): 91-102. doi: 10.3969/j.issn.0253-4193.2014.12.009

Oil fingerprinting of polyaromatic hydrocarbons applied to the identification study of oil spill from ship

doi: 10.3969/j.issn.0253-4193.2014.12.009
  • Received Date: 2014-05-19
  • Rev Recd Date: 2014-06-25
  • Differences in the nature of fuel oil and crude oil which are main oil types in marine oil spill determine the different identification methods,so it is significative to seek a suitable method for oil spill identification from the ship. The comparative oil fingerprinting characteristic analysis of polyaromatic hydrocarbons between the spilled oil samples and the suspected oils from ships had been carried on using gas chromatography/mass spectrometry(GC/MS) as a primary analysis method after the samples were separated by the column chromatography method,and the oil source was traced successfully in the oil spill from the ship took place in Pearl River estuary by inner component triangular diagram and cluster analysis based on aromatic hydrocarbon parameters. The results showed that the aromatic oil fingerprinting of the sample from the fourth ship was the most similar with the spilled oil sample,so the oil spill was caused by the fourth ship. The characteristic of aromatic compounds is the main evidence of these weathered oil spill identification because the aromatics were of higher levels and richer variety than saturated hydrocarbons. The key was that the different behavior performed by the organic molecules in oils after undergoing weathering should be fully considered when using oil fingerprinting parameters for the oil spill identification. So,the oil fingerprinting of polyaromatic hydrocarbons are effective for identification of oil spill from the ship.
  • loading
  • Wang Z D,Fingas M,Page D S. Oil spill identification[J]. Journal of Chromatography A,1999,843(1/2): 369-411.
    Sammarco P W,Kolian S R,Warby R A F,et al. Distribution and concentrations of petroleum hydrocarbons associated with the BP/Deepwater Horizon Oil Spill,Gulf of Mexico[J]. Marine Pollution Bulletin,2013,73(1): 129-143.
    Wang C Y,Chen B,Zhang B Y,et al. Fingerprint and weathering characteristics of crude oils after Dalian oil spill,China[J]. Marine Pollution Bulletin,2013,71(1/2): 64-68.
    孙培艳,高振会,崔文林,等. 油指纹鉴别技术发展及应用[M]. 北京: 海洋出版社,2007: 9-11.
    Wang Z D,Stout S A,Fingas M. Forensic fingerprinting of biomarkers for oil spill characterization and source identification[J]. Environmental Forensics,2006,7(2): 105-146.
    Munoz D,Guiliano M,Doumenq P,et al. Long term evolution of petroleum biomarkers in mangrove soil[J]. Marine Pollution Bulletin,1997,34(11): 868-874.
    Wang Z D,Stout S A. Oil Spill Environmental Forensics: Fingerprinting and Source Identification[M]. Boston: Academic Press,2006.
    Wang Z D,Yang C,Yang Z,et al. Forensic fingerprinting and source identification of the 2009 Sarnia (Ontario) oil spill[J]. Journal of Environmental Monitoring,2011,13(11): 3004-3017.
    Yim U H,Ha S Y,An J G,et al. Fingerprint and weathering characteristics of stranded oils after the Hebei Spirit oil spill[J]. Journal of Hazardous Materials,2011,197: 60-69.
    Barakat A O,Mostafa A R,Rullkötter J,et al. Application of a multimolecular marker approach to fingerprint petroleum pollution in the marine environment[J]. Marine Pollution Bulletin,1999,38(7): 535-544.
    Wang Z D,Fingas M F. Development of oil hydrocarbon fingerprinting and identification techniques[J]. Marine Pollution Bulletin,2003,47(9/12): 423-452.
    徐恒振. 灰色关联度聚类分析在溢油鉴别中的应用[J]. 中国环境科学,1995,15(1): 22-28.
    Salas N,Ortiz L,Gilcoto M,et al. Fingerprinting petroleum hydrocarbons in plankton and surface sediments during the spring and early summer blooms in the Galician coast(NW Spain)after the Prestige oil spill[J]. Marine Environmental Research,2006,62(5): 388-413.
    赵玉慧,孙培艳,王鑫平,等. 多环芳烃指纹用于渤海采油平台原油的鉴别[J]. 色谱,2008,26(1): 43-49.
    Wang Z D,Fingas M F,Li K. Fractionation of a light crude oil and identification and quantitation of aliphatic,aromatic,and biomarker compounds by GC-FID and GC-MS,Part II[J]. Journal of Chromatographic Science,1994,32(9): 367-382.
    Daling P S,Faksness L G,Hansen A B,et al. Improved and standardized methodology for oil spill fingerprinting[J]. Environmental Forensics,2002,3(3): 263-278.
    刘星,王震,马新东,等. 柴油的指纹提取及基于其指纹信息的层次聚类分析[J]. 环境污染与防治,2011,33(12): 18-22.
    王传远,胡晓珂. 燃料油的重度风化规律及其在溢油鉴定中的应用研究 //中国海洋湖沼学会第十次全国会员代表大会暨学术研讨会论文集. 中国海洋湖沼学会,2012.
    徐世平,孙永革. 一种适用于沉积有机质族组分分离的微型柱色谱法[J]. 地球化学,2006,35(6): 681-688.
    Kaplan I R,Galperin Y,Lu S T,et al. Forensic Environmental Geochemistry: differentiation of fuel-types,their sources and release time[J]. Organic Geochemistry,1997,27(5/6): 289-299,301-317.
    Mansuy L,Philp R P,Allen J,et al. Source identification of oil spills based on the isotopic composition of individual components in weathered oil samples[J]. Environmental Science and Technology,1997,31(12): 3417-3425.
    Ebrahimi D,Li J F,Hibbert D B. Classification of weathered petroleum oils by multi-way analysis of gas chromatography-mass spectrometry data using PARAFAC2 parallel factor analysis[J]. Journal of Chromatography A,2007,1166(1/2): 163-170.
    Garrett R M,Pickering I J,Haith C E,et al. Photooxidation of crude oils[J]. Environmental Science and Technology,l998,32: 3719-3723.
    Dutta T K,Harayama S. Fate of crude oil by the combination of photooxidation and biodegradation[J]. Environmental Science and Technology,2000,34(8): 1500-l505.
    Christensen J H,Hansen A B,Karlson U,et al. Multivariate statistical methods for evaluating biodegradation of mineral oil[J]. Journal of Chromatography A,2005,1090: 133-145.
    Radke M. Application of aromatic compounds as maturity indicators in source rocks and crude oils[J]. Marine and Petroleum Geology,1988,5(3): 224-236.
    Santamaría-Orozco D,Horsfield B,Di Primio R,et al. Influence of maturity on distributions of benzo-and dibenzothiophenes in Tithonian source rocks and crude oils,Sonda de Campeche,Mexico[J]. Organic Geochemistry,1988,28(7/8): 423-439.
    Chakhmakhchev A,Suzuki M,Takayama K,et al. Distribution of alkylated dibenzothiophenes in petroleum as a tool for maturity assessments[J]. Organic Geochemistry,1997,26(7/8): 483-489.
    Radke M,Willsch H,Leythaeuser D,et al. Aromatic components of coal: Relation of distribution pattern to rank[J]. Geochimica et Cosmochimica Acta,1982,46(10): 1831-1848.
    Angelin M L,Collignan A,Bellocq J,et al. Investigation of polycyclic aromatic hydrocarbons in source rock bitumens and petroleums by high pressure liquid chromatography[J]. Comptes Rendues de 'l Academie des Sciences Paris,Series Ⅱ,1983,296: 705-708.
    Mackenzie A S. Application of biological marker in petroleum geochemistry[M]//Brooks J,Welte D H. Advances in Petroleum Geochemistry. London: Academic Press,1984: 115-214.
    包建平,王铁冠,王金渝. 下扬子地区海相中、古生界有机地球化学[M]. 重庆: 重庆大学出版社,1996: 104.
    Chakhmakhchev A,Suzuki N. Saturate biomarkers and aromatic sulfur compounds in oils and condensates from different source rock lithologies of Kazakhstan,Japan and Russia[J]. Organic Geochemistry,1995,23(4): 289-299.
  • 加载中

Catalog

    通讯作者: 陈斌, bchen63@163.com
    • 1. 

      沈阳化工大学材料科学与工程学院 沈阳 110142

    1. 本站搜索
    2. 百度学术搜索
    3. 万方数据库搜索
    4. CNKI搜索
    Article views (1252) PDF downloads(1132) Cited by()
    Proportional views
    Related

    /

    DownLoad:  Full-Size Img  PowerPoint
    Return
    Return