Message Board

Respected readers, authors and reviewers, you can add comments to this page on any questions about the contribution, review, editing and publication of this journal. We will give you an answer as soon as possible. Thank you for your support!

Full name
E-mail
Phone number
Title
Message
Verification Code
Chen Xin, Song Jinming, Yuan Huamao, Li Xuegang, Li Ning, Duan Liqin, Qu Baoxiao. CO2 fluxes across the air-sea interface of the East China Sea in summer 2012 and the change tendency of regional carbon sink strength[J]. Haiyang Xuebao, 2014, 36(12): 18-31. doi: 10.3969/j.issn.0253-4193.2014.12.002
Citation: Chen Xin, Song Jinming, Yuan Huamao, Li Xuegang, Li Ning, Duan Liqin, Qu Baoxiao. CO2 fluxes across the air-sea interface of the East China Sea in summer 2012 and the change tendency of regional carbon sink strength[J]. Haiyang Xuebao, 2014, 36(12): 18-31. doi: 10.3969/j.issn.0253-4193.2014.12.002

CO2 fluxes across the air-sea interface of the East China Sea in summer 2012 and the change tendency of regional carbon sink strength

doi: 10.3969/j.issn.0253-4193.2014.12.002
  • Received Date: 2014-01-07
  • Rev Recd Date: 2014-05-02
  • The surface water partial pressure of CO2(pCO2),dissolved inorganic carbon(DIC),dissolved organic carbon(DOC) and particulate organic carbon(POC) in the East China Sea(ECS) were investigated during the survey in July 2012. The results showed that the adjacent area of the Changjiang estuary had higher DOC and POC contents and lower DIC than the southern shelf. Surface pCO2 in the ECS ranged from 96.28 to 577.7 μatm (mean is 297.6 μatm,1 atm is 101 325 Pa). Low pCO2 levels were found in area (30°-33°N,123°-125°E) of the Changjiang Diluted Water (CDW),whereas high pCO2 levels occurred in the southern ECS shelf affected by the Taiwan Current Warm. The surface pCO2 was mainly influenced by the Changjiang freshwater input and mixing,Taiwan warm current water and biological production. The average summer FCO2 in the ECS was(-6.410±7.486) mmol/(m2·d),indicating that the ECS served as a CO2 sink which absorbed (1.83±1.98)×104 t carbon every day in the summer. The regional carbon fluxes sorted from high to low as CDW,YEMW,SMW,CUW(Coastal Upwelling Water) and TWCW. Comparing with the historical data,the effect of the ECS as a CO2 sink was gradually enhancing in the last ten years. The CDW was the biggest contributor to the increased carbon sink in the ECS. And the FCO2 annual growth rate in the CDW area was -0.814 mmol/(m2·d),meaning that every summer the CDW could take up 5.46×104 t more than last year's.
  • loading
  • Frankignoulle M,Borges A V. European continental shelf as a significant sink for atmospheric carbon dioxide[J]. Global Biogeochemical Cycles,2001,15(3): 569-576.
    Chen C T A,Liu C T,Chuang W S,et al. Enhanced buoyancy and hence upwelling of subsurface Kuroshio waters after a typhoon in the southern East China Sea[J]. Journal of Marine Systems,2003,42(1/2): 65-79.
    Chen C T A,Borges A V. Reconciling opposing views on carbon cycling in the coastal ocean: Continental shelves as sinks and near-shore ecosystems as sources of atmospheric CO2[J]. Deep-Sea Research Part Ⅱ: Topical Studies in Oceanography,2009,56(8/10): 578-590.
    Cai W J. Estuarine and coastal ocean carbon paradox: CO2 sinks or sites of terrestrial carbon incineration?[J]. Annual Review of Marine Science,2011,3: 123-145.
    Dai M H,Cao Z M,Guo X H,et al. Why are some marginal seas sources of atmospheric CO2?[J]. Geophysical Research Letters,2013,40(10): 2154-2158.
    Cai W J,Dai M H,Wang Y C. Air-sea exchange of carbon dioxide in ocean margins: A province-based synthesis[J]. Geophysical Research Letters,2006,33(12): L12603.
    宋金明,徐永福,胡维平,等. 中国近海与湖泊碳的生物地球化学[M]. 北京: 科学出版社,2008: 63-226.
    Chen C T A,Huang T H,Chen Y C,et al. Air-sea exchanges of CO2 in the world's coastal seas[J]. Biogeosciences,2013,10: 6509-6544.
    曲宝晓,宋金明,袁华茂,等. 东海海-气界面二氧化碳通量的季节变化与控制因素研究进展[J]. 地球科学进展,2013,28(7): 783-793.
    Tsunogai S,Watanabe S,Sato T. Is there a "continental shelf pump" for the absorption of atmospheric CO2?[J]. Tellus B,1999,51(3): 701-712.
    张龙军,王彬宇,张经. 东海冬、夏两季表层海水的二氧化碳分压[J]. 青岛海洋大学学报,1999,29(增刊): 149-153.
    Wang S L,Chen C T A,Hong G H,et al. Carbon dioxide and related parameters in the East China Sea[J]. Continental Shelf Research,2000,20(4/5): 525-544.
    张龙军. 东海海-气界面CO2通量研究[D]. 青岛: 中国海洋大学,2003: 87-89.
    谭燕,张龙军,王凡,等. 夏季东海西部表层海水中的pCO2及海-气界面通量[J]. 海洋与湖沼,2004,35(3): 239-245.
    Shim J H,Kim D,Kang Y C,et al. Seasonal variations in pCO2 and its controlling factors in surface seawater of the northern East China Sea[J]. Continental Shelf Research,2007,27(20): 2623-2636.
    刘建栋. 冬季东中国海表层pCO2的分布特征及控制因素分析[D]. 青岛: 中国海洋大学,2008: 46-51.
    Chou W C,Gong G C,Sheu D D,et al. Surface distributions of carbon chemistry parameters in the East China Sea in summer 2007[J]. Journal of Geophysical Research,2009,114(C7): C07026.
    Chou W C,Gong G C,Tseng C M,et al. The carbonate system in the East China Sea in winter[J]. Marine Chemistry,2011,123(1/4): 44-55.
    Tseng C M,Liu K K,Gong G C,et al. CO2 uptake in the East China Sea relying on Changjiang runoff is prone to change[J]. Geophysical Research Letters,2011,38(24).
    朱连磊,宋金明,李学刚,等. 东海中北部海域秋季表层海水中无机碳与海气界面碳的迁移[J]. 海洋科学,2012,36(10): 26-32.
    Kim D,Choi S H,Shim J H,et al. Revisiting the Seasonal Variations of Sea-Air CO2 Fluxes in the Northern East China Sea[J]. Terrestrial,Atmospheric & Oceanic Sciences,2013,24(3).
    Qu B X,Song J M,Li X G,et al. pCO2 distribution and CO2 flux on the inner continental shelf of the East China Sea during summer 2011[J]. Chinese Journal of Oceanology and Limnology,2013,31(5): 1088-1097.
    林晶. 长江口及其毗邻海区溶解有机碳和颗粒有机碳的分布[D]. 上海: 华东师范大学,2007: 17-74.
    Dickson A G,Sabine C L,Christian J R. Guide to best practices for ocean CO2 measurements[D]. PICES Special Publication 3,2007: 191.
    Pierrot D,Lewis E,Wallace D W R. MS Excel program developed for CO2 system calculations. ORNL/CDIAC-105[D]. Carbon Dioxide Information Analysis Center,Oak Ridge National Laboratory,US Department of Energy,Oak Ridge,Tennessee,2006.
    Mehrbach C,Culberson C H,Hawley J E,et al. Measurement of the apparent dissociation constants of carbonic acid in seawater at atmospheric pressure[J]. Limnology and Oceanography,1973,18(6): 897-907.
    Dickson A G,Millero F J. A comparison of the equilibrium constants for the dissociation of carbonic acid in seawater media[J]. Deep Sea Research Part A. Oceanographic Research Papers,1987,34(10): 1733-1743.
    Hoppe C J M,Langer G,Rokitta S D,et al. On CO2 pertubation experiments: over-determination of carbonate chemistry reveals inconsistencies[J]. Biogeosciences Discussions,2010,7: 1707-1726.
    Chai C,Yu Z M,Shen Z L,et al. Nutrient characteristics in the Yangtze River Estuary and the adjacent East China Sea before and after impoundment of the Three Gorges Dam[J]. Science of the Total Environment,2009,407(16): 4687-4695.
    Weiss R F. Carbon dioxide in water and seawater: the solubility of a non-ideal gas[J]. Marine Chemistry,1974,2(3): 203-215.
    Takahashi T,Sutherland S C,Sweeney C,et al. Global sea-air CO2 flux based on climatological surface ocean pCO2,and seasonal biological and temperature effects[J]. Deep-Sea Research Part Ⅱ: Topical Studies in Oceanography,2002,49(9/10): 1601-1622.
    Weiss R F,Price B A. Nitrous oxide solubility in water and seawater[J]. Marine Chemistry,1980,8(4): 347-359.
    Wanninkhof R. Relationship between wind speed and gas exchange over the ocean[J]. Journal of Geophysical Research: Oceans (1978—2012),1992,97(C5): 7373-7382.
    Lee H J,Chao S Y. A climatological description of circulation in and around the East China Sea[J]. Deep-Sea Research Part Ⅱ: Topical Studies in Oceanography,2003,50(6/7): 1065-1084.
    Gong G C,Lee Chen Y L,Liu K K. Chemical hydrography and chlorophyll a distribution in the East China Sea in summer: implications in nutrient dynamics[J]. Continental Shelf Research,1996,16(12): 1561-1590.
    Hellings L,Dehairs F,Van Damme S,et al. Dissolved inorganic carbon in a highly polluted estuary (the Scheldt)[J]. Limnology and Oceanography,2001,46(6): 1406-1414.
    高学鲁,宋金明,李学刚,等. 长江口及杭州湾邻近海域夏季表层海水中的溶解无机碳[J]. 海洋科学,2008,32(4): 61-67.
    Zweifel U L,Wikner J,Hagström A,et al. Dynamics of dissolved organic carbon in a coastal ecosystem[J]. Limnology and Oceanography,1995,40(2): 299-305.
    张乃星,宋金明,贺志鹏. 海水颗粒有机碳(POC)变化的生物地球化学机制[J]. 生态学报,2006,26(7): 2328-2339.
    曹知勉. 南海无机碳代谢及其在碳循环中的作用初探[D]. 厦门: 厦门大学,2008: 25-31.
    Sackett W M,Moore W S. Isotopic variations of dissolved inorganic carbon[J]. Chemical Geology,1966,1: 323-328.
    Bakker D C E,de Baar H J W,de Wilde H P J. Dissolved carbon dioxide in Dutch coastal waters[J]. Marine Chemistry,1996,55(3/4): 247-263.
    Chen C T A,Zhai W D,Dai M H. Riverine input and air-sea CO2 exchanges near the Changjiang (Yangtze River) Estuary: Status quo and implication on possible future changes in metabolic status[J]. Continental Shelf Research,2008,28(12): 1476-1482.
    Zhai W D,Dai M H. On the seasonal variation of air-sea CO2 fluxes in the outer Changjiang (Yangtze River) Estuary,East China Sea[J]. Marine Chemistry,2009,117(1/4): 2-10.
    Chen C T A,Huang T H,Fu Y H,et al. Strong sources of CO2 in upper estuaries become sinks of CO2 in large river plumes[J]. Current Opinion in Environmental Sustainability,2012,4(2): 179-185.
    Cai W J,Dai M H,Wang Y C,et al. The biogeochemistry of inorganic carbon and nutrients in the Pearl River estuary and the adjacent Northern South China Sea[J]. Continental Shelf Research,2004,24(12): 1301-1319.
    Chen F Z,Cai W J,Benitez-Nelson C,et al. Sea surface pCO2-SST relationships across a cold-core cyclonic eddy: Implications for understanding regional variability and air-sea gas exchange[J]. Geophysical Research Letters,2007,34(10).
    文斐,孙晓霞,郑珊,等. 2011年春、夏季黄、东海叶绿素a和初级生产力的时空变化特征[J]. 海洋与湖沼,2012,43(3): 438-444.
    Li X G,Song J M,Niu L F,et al. Role of the Jiaozhou Bay as a source/sink of CO2 over a seasonal cycle[J]. Scientia Marina,2007,71(3): 441-450.
    中华人民共和国水利部. 中国河流泥沙公报(2003-2011)[D]. 2004-2012.
    Xu K H,Milliman J D,Yang Z S,et al. Climatic and anthropogenic impacts on water and sediment discharges from the Yangtze River (Changjiang),1950—2005[M]//Large Rivers: Geomorphology and Management. Chichester,UK: John Wiley & Sons,2007: 609-626.
    Yang Z S,Wang H,Saito Y,et al. Dam impacts on the Changjiang (Yangtze) River sediment discharge to the sea: The past 55 years and after the Three Gorges Dam[J]. Water Resources Research,2006,42(4).
    Cai W J,Chen L,Chen B,et al.Decrease in the CO2 uptake capacity in an ice-free Arctic Ocean basin[J].Science,2010,329(5991):556-559.
  • 加载中

Catalog

    通讯作者: 陈斌, bchen63@163.com
    • 1. 

      沈阳化工大学材料科学与工程学院 沈阳 110142

    1. 本站搜索
    2. 百度学术搜索
    3. 万方数据库搜索
    4. CNKI搜索
    Article views (1616) PDF downloads(1417) Cited by()
    Proportional views
    Related

    /

    DownLoad:  Full-Size Img  PowerPoint
    Return
    Return