镭、氡同位素示踪调水调沙对黄河口水体运移及营养盐分布特征的影响

张晓洁; 许博超; 夏冬; 江雪艳; 简慧敏

doi:10.3969/j.issn.0253-4193.2016.08.004

镭、氡同位素示踪调水调沙对黄河口水体运移及营养盐分布特征的影响

doi: 10.3969/j.issn.0253-4193.2016.08.004

1.
中国海洋大学海洋化学理论与工程教育部重点实验室, 山东青岛 266100;海洋国家实验室海洋生态与环境科学功能实验室, 山东青岛 266071;中国海洋大学化学化工学院, 山东青岛 266100
2.
中国海洋大学环境科学与工程学院, 山东青岛 266100;中国科学院生态环境研究中心, 北京 100085
3.
中国海洋大学海洋化学理论与工程教育部重点实验室, 山东青岛 266100

基金项目: 国家自然科学基金（41576075，41206064，41376085）；山东省自然科学基金（ZR2012DQ002）；青岛市科技计划基础研究项目（13-1-4-224-jch）。

计量
- 文章访问数: 1210
- HTML全文浏览量: 11
- PDF下载量: 951
- 被引次数: 0
出版历程
- 收稿日期: 2015-12-19
- 修回日期: 2016-02-19

Using natural radium and radon isotopes trace the water transport process and nutrients distribution in the Yellow River Estuary under the influence of the Water-Sediment Regulation Scheme

1.
Key Laboratory of Marine Chemistry Theory and Technology, Ministry of Education, Ocean University of China, Qingdao 266100, China;Laboratory for Marine Ecology and Environmental Science, Qingdao National Laboratory for Marine Science and Technology, Qingdao 266071, China;College of Chemistry and Chemical Engineering, Ocean University of China, Qingdao 266100, China
2.
College of Environmental Science and Engineering, Ocean University of China, Qingdao 266100, China;Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences, Beijing 100085, China
3.
Key Laboratory of Marine Chemistry Theory and Technology, Ministry of Education, Ocean University of China, Qingdao 266100, China

摘要

摘要: 为研究调水调沙影响下的镭、氡同位素和营养盐在黄河口的分布特征，于2013年7月调水调沙期间在黄河口及其邻近海域进行了多点的连续观测。研究发现：(1)黄河口海域镭、氡同位素分布呈现明显的“分区”现象，南北两区分别为“调水调沙影响非显著区域”和“调水调沙影响显著区域”，北部海域镭、氡同位素浓度高值主要来源于陆源输入(包括河流输入和海底地下水排放)；(2)调查期间，北部海域水体年龄为(2.9±1.6)d，南部海域水体年龄为(5.0±2.1)d；水龄随潮汐变化表现出涨潮时水龄增大、落潮时水龄减小的波动趋势；(3)北部海域溶解无机氮(DIN)和溶解硅(DSi)含量明显高于南部海域，而溶解无机磷(DIP)在两个区域的含量相差不大。
- 黄河口 /
- 调水调沙 /
- 镭同位素 /
- 氡同位素 /
- 营养盐
Abstract: In order to study the distribution of radium isotopes, radon isotopes and nutrients under the influence of the Water-Sediment Regulation Scheme (WSRS) in the Yellow River Estuary. We carried out 24 h time-series observations at several stations in the estuary and coastal areas in July 2013. The results indicate that: (1) the distributions of radium isotopes and radon isotopes at south side were both different from which in the north side of the estuary, leading the estuary to be divided into two zones. The north zone was under a remarkable influence of WSRS and the south zone was under little influence of WSRS, respectively. High concentrations of radium and radon isotopes in the north zone were mainly due to terrestrial input, such as river discharge and submarine groundwater discharge. (2) Water ages in the north zone was (2.9±1.6)d, which in the south zone was (5.0±2.1)d. Water ages increased with rising tide and decreased with falling tide. (3) Dissolved inorganic nitrogen (DIN) and dissolved silicate (DSi) distribution also showed zonation characteristics, which concentrations were significantly higher in north area. The concentrations of dissolved inorganic phosphorus (DIP), however, were not distinct in the whole study area.
- Yellow River Estuary /
- Water-Sediment Regulation Scheme /
- radium isotope /
- radon isotope /
- nutrients

HTML全文

参考文献(27)

毕乃双, 杨作升, 王厚杰, 等. 黄河调水调沙期间黄河入海水沙的扩散与通量[J]. 海洋地质与第四纪地质, 2010(2):27-34. Bi Naishuang, Yang Zuosheng, Wang Houjie, et al. Characteristics of dispersal of the Yellow River water and sediment to the sea during Water-Sediment Regulation period of the Yellow River and its dynamic mechanism[J]. Marine Geology & Quaternary Geology, 2010(2):27-34.

王玉成. 黄河调水影响下河口区盐度分布的观测与模拟研究[D]. 青岛:中国海洋大学, 2010. Wang Yucheng. Study on response of salinity distribution around the Yellow River mouth to abrupt change in river discharge with in situ observation and numerical simulation[D]. Qingdao:Ocean University of China, 2010.

姚庆祯, 于志刚, 王婷, 等. 调水调沙对黄河下游营养盐变化规律的影响[J]. 环境科学, 2009, 30(12):3534-3540. Yao Qingzhen, Yu Zhigang, Wang Ting, et al. Effect of the first Water-Sediment Regulation on the variations of dissolved inorganic nutrients' concentrations and fluxes in the lower main channel of the Yellow River[J]. Environmental Science, 2009, 30(12):3534-3540.

Wang H J, Yang Z S, Bi N S, et al. Rapid shifts of the river plume pathway off the Huanghe (Yellow) River mouth in response to Water-Sediment Regulation Scheme in 2005[J]. Chinese Science Bulletin, 2005, 50(24):2878-2884.

Veeh H H, Moore W S, Smith S V. The behaviour of uranium and radium in an inverse estuary[J]. Continental Shelf Research, 1995, 15(13):1569-1583.

Moore W S, Arnold R. Measurement of ²²³Ra and ²²⁴Ra in coastal waters using a delayed coincidence counter[J]. Journal of Geophysical Research, 1996, 101(C1):1321-1329.

Waska H, Kim S, Kim G, et al. An efficient and simple method for measuring ²²⁶Ra using the scintillation cell in a delayed coincidence counting system (RaDeCC)[J]. Journal of Environmental Radioactivity, 2008, 99(12):1859-1862.

Lambert M J, Burnett W C. Submarine groundwater discharge estimates at a Florida coastal site based on continuous radon measurements[J]. Biogeochemistry, 2003, 66(1/2):55-73.

Xu B C, Xia D, Burnett W C, et al. Natural ²²²Rn and ²²⁰Rn indicate the impact of the Water-Sediment Regulation Scheme (WSRS) on submarine groundwater discharge in the Yellow River estuary, China[J]. Applied Geochemistry, 2014, 51:79-85.

Schubert M, Paschke A, Lieberman E, et al. Air-water partitioning of ²²²Rn and its dependence on water temperature and salinity[J]. Environmental Science & Technology, 2012, 46(7):3905-3911.

Grasshoff K, Kremling K, Ehrhardt M. Methods of Seawater Analysis[M]. 3rd ed. New York:John Wiley & Sons, 1999.

Xia D, Yu Z G, Xu B C, et al. Variations of hydrodynamics and submarine groundwater discharge in the Yellow River estuary under the influence of the Water-Sediment Regulation Scheme[J]. Estuaries and Coasts, 2016, 39(2):333-343.

Li Y H, Chan L H. Desorption of Ba and ²²⁶Ra from river-borne sediments in the Hudson estuary[J]. Earth and Planetary Science Letters, 1979, 43(3):343-350.

Dulaiova H, Burnett W C. Evaluation of the flushing rates of Apalachicola Bay, Florida via natural geochemical tracers[J]. Marine Chemistry, 2008, 109(3/4):395-408.

Moore W S. Large groundwater inputs to coastal waters revealed by ²²⁶Ra enrichments[J]. Nature, 1996, 380(6575):612-614.

Swarzenski P W, Reich C, Kroeger K D, et al. Ra and Rn isotopes as natural tracers of submarine groundwater discharge in Tampa Bay, Florida[J]. Marine Chemistry, 2007, 104(1/2):69-84.

Charette M A, Moore W S, Burnett W C. Uranium-and thorium-series nuclides as tracers of submarine groundwater discharge[J]. Radioactivity in the Environment, 2008, 13:155-191.

Peterson R N, Burnett W C, Taniguchi M, et al. Radon and radium isotope assessment of submarine groundwater discharge in the Yellow River delta, China[J]. Journal of Geophysical Research, 2008, 113(C9):C09021.

Taniguchi M, Ishitobi T, Chen J Y, et al. Submarine groundwater discharge from the Yellow River delta to the Bohai Sea, China[J]. Journal of Geophysical Research, 2008, 113(C6):C06025.

Xu B C, Burnett W, Dimova N, et al. Hydrodynamics in the Yellow River Estuary via radium isotopes:ecological perspectives[J]. Continental Shelf Research, 2013, 66:19-28.

Moore W S. Ages of continental shelf waters determined from ²²³Ra and ²²⁴Ra[J]. Journal of Geophysical Research, 2000, 105(C9):22117-22122.

Moore W S, Krest J. Distribution of ²²³Ra and ²²⁴Ra in the plumes of the Mississippi and Atchafalaya Rivers and the Gulf of Mexico[J]. Marine Chemistry, 2004, 86(3/4):105-119.

孙效功, 杨作升, 陈彰榕. 现行黄河口海域泥沙冲淤的定量计算及其规律探讨[J]. 海洋学报, 1993, 15(1):129-136. Sun Xiaogong, Yang Zuosheng, Chen Zhangrong. Quantitative calculation and law discussing for sediment erosion and siltation in river mouth of Yellow River[J]. Haiyang Xuebao, 1993, 15(1):129-136.

张向上. 黄河口碳输运过程及其对莱州湾的影响[D]. 青岛:中国海洋大学, 2007. Zhang Xiangshang. The transport of inorganic and organic carbon in the Yellow River estuary and its effect on Laizhou Bay[D]. Qingdao:Ocean University of China, 2007.

于立霞, 简慧敏, 王兆锟, 等. 夏季辽河口各形态营养盐的河口混合行为[J]. 海洋科学, 2011, 35(12):68-74. Yu Lixia, Jian Huimin, Wang Zhaokun, et al. The mixing behavior of nutrients in summer at Liaohe Estuary[J]. Marine Sciences, 2011, 35(12):68-74.

石晓勇, 史致丽. 黄河口磷酸盐缓冲机制的探讨Ⅲ.磷酸盐交叉缓冲图及"稳定pH范围"[J]. 海洋与湖沼, 2000, 31(4):441-447. Shi Xiaoyong, Shi Zhili. Discussion of phosphate buffer mechanism in Huanghe river estuary Ⅲ. Cross over buffer plot of phosphate and "stable pH range"[J]. Oceanologia et Limnologia Sinica, 2000, 31(4):441-447.

张正斌, 陈镇东, 刘莲生, 等. 海洋化学原理和应用——中国近海的海洋化学[M]. 北京:海洋出版社, 1999. Zhang Zhengbin, Chen Zhendong, Liu Liansheng, et al. Principles and Applications of Marine Chemistry-China's Offshore Marine Chemistry[M]. Beijing:China Ocean Press, 1999.

施引文献

资源附件(0)

访问统计